Based on Eq. (1), the carbon emissions of cultivated land use in China from 1991 to 2021 are calculated, and the temporal variation characteristics of carbon emissions and growth rate of cultivated land use in China can be obtained (Fig. 2). The results show that the carbon emissions of cultivated land use in China have a rising and then declining trend, increasing from 36.9707 million tons in 1991 to 69.7625 million tons in 2021, with an average annual increase of 1.1273 million tons and an average annual growth rate of 2.23%; which may be due to the increase in the input of agricultural materials such as fertilizers, pesticides, agricultural films, and agricultural machinery or the degree of soil destruction caused by agricultural chemical and mechanization, together increasing carbon emissions of cultivated land use. Among them, the average annual growth rates of fertilizer, pesticide, agricultural film, agricultural machinery, tillage, and agricultural irrigation are 2.12%, 1.78%, 3.86%, 0.56%, 0.41%, and 1.24%, respectively. However, the growth rate declined after 2010 and stepped into a negative growth stage in 2016. The total carbon emission of cultivated land use decreased by 3.71% and 4.06% in 2018 and 2019, respectively, indicating that the carbon emission of cultivated land use in China is effectively controlled; this could be due to the continuous practice of the concept of low-carbon green development in agricultural production since the 18th CPC National Congress, since when China's cultivated land use pattern is changing from high-carbon to low-carbon.
The spatial patterns of carbon emissions from cultivated land use in 31 provinces of mainland China in 1991, 2000, 2010, and 2020 can be obtained with the calculation above. In order to compare the variability of carbon emissions of cultivated land use inter-provinces and regions more intuitively, the natural discontinuity method was used to divide carbon emissions into five levels; that is, level 1 has the lowest carbon emissions, and level 5 has the highest carbon emissions; as shown in Fig. 3.
At the provincial level, the provinces with level 1 and level 2 carbon emissions tend to decrease. Nine provinces, including Tibet, Ningxia, and Qinghai, belonged to the level 1 carbon emission region in 1991, and by 2021, two provinces were reduced. The level 2 carbon emission region was reduced from twelve provinces, including Shanxi, Guizhou, Zhejiang, and Fujian, to seven provinces in 2010 (Heilongjiang, Jilin, Liaoning, and Shaanxi provinces changed from level 2 carbon emission region to level 3 carbon emission region), and to six provinces in 2021 (Gansu Province turns to level 3 carbon emission region). From 1991 to 2021, two new provinces, Henan and Shandong, were added as Level 5 carbon emission provinces, and five new provinces, Hebei, Hubei, Anhui, Jiangsu, and Xinjiang, were added as Level 4 carbon emission provinces.
The above conclusions show that the traditional major grain-producing provinces are dominated by planting and highly dependent on cultivated land. At the same time, more inputs of high-carbon materials such as fertilizers, agricultural films, and pesticides lead to high carbon emissions from cultivated land use. These provinces have be-come the primary source of carbon emissions from cultivated land use, and the inter-provincial differences in carbon emissions tend to expand. At the regional level, the provinces with higher carbon emissions are mainly concentrated in the central and eastern regions, possibly due to the higher degree of intensification of cultivated land use in these regions. Compared with the difference in carbon emissions in different regions in 1991, the difference in carbon emissions in different regions tends to shrink. However, the total carbon emissions show a shift from the characteristics of "western region > northeastern region > eastern region > central region" in 1991, "eastern region > central region > western region > northeastern region" in 2000 and 2010, to "western region > central region > eastern region > northeastern region" in 2021.
In terms of sub-regions, from 1991 to 2021, the average annual carbon emissions from cultivated land use in 13 major grain-producing provinces in China, including Heilongjiang, Henan, Shandong, Anhui, Jilin, and Hebei, were 42.6548 million tons, much higher than the remaining non-major grain-producing provinces of 20.5335 million tons. China should focus on transforming agricultural production methods in major grain-producing areas, widely adopting energy-saving and emission-reduction technologies, and comprehensively improving the utilization efficiency of agricultural materials to realize the carbon emission-reduction of cultivated land use eventually.