Past studies have highlighted that SAI can affect the mean climate of the stratosphere 28,46,47. Sulfate aerosols located in the stratosphere are effective at reflecting and scattering incoming solar radiation and, therefore, act to cool the surface and the free troposphere, but also absorb infrared radiation 48, resulting in a warming of the lower tropical stratosphere 46,49,50. In the specific SAI scenario used here, 30–40 Tg-SO2/yr injections were needed to counter the RCP8.5 warming of 3–4 degrees C by 2070–2090 in this model. The resulting lower stratospheric warming that maximizes in the tropics reaches more than > 8 degrees Celsius at ~ 50 hPa (Fig. 2a).
The strong anomalous warming of the lower stratosphere imposed by SAI leads to tropical tropospheric circulation changes 32,47,51, a weakening of the subtropical jets in both hemispheres (Fig. 2b) and a modification in the wave activity in the subtropics (Fig. 2c). Independently of SAI, previous studies have linked upper tropospheric waves to Indian and Asian monsoons 44,52,53, whereby summertime planetary wave activity at ~ 200 hPa across Indian longitudes strongly correlates with SAM rainfall 54–56. Here, we identify a similar connection between the 200 hPa meridional wind anomalies and rainfall changes. SAI-induced lower stratospheric heating and weakening of the northern subtropical jet modulate the mean summertime 200 hPa meridional winds (Fig. 2c), with the anomalies resembling a structure similar to the stationary Rossby wave 44,56. The meridional wind response to SAI in the South Asian region basically reinforces the climatological wave pattern (Fig. S2) and results in an anomalous cyclonic circulation at 200 hPa, which consists of anomalous southward flow to the west of India and anomalous poleward flow to the east of India (Fig. 2c). The positive anomaly of the 200 hPa meridional winds is aligned with the reduction in rainfall over the central and northern parts of India.
These changes are also aligned with changes in the climatological Asian Summer Monsoon Anticyclone (ASMA) in the upper troposphere (Figure S3a) that forms across the Asian Summer Monsoon region and is linked to the heating of the Tibetan plateau and deep convective activities over the head of the Bay of Bengal 57.
Under SAI, the ASMA decelerates, which is illustrated by the anomalously cyclonic flow compared to the control simulation (Fig. 2d). We also observe an anomalous splitting of ASMA into two parts, one over India and the other over the Middle East and North Africa region (Fig. 2d). The deceleration of ASMA contributes to the reduction in the strength of the summer monsoon circulation in the lower troposphere (Fig. 2e; see Fig. S3b for the climatology) and the simulated SAI-induced drying over central and northern India.
The changes in the upper atmospheric wave activities and weakening of ASMA are also reflected in the associated changes in vertical velocities (Fig. 2f). Changes in the large-scale vertical motions often indicate the surface pressure patterns. For example, anomalous sinking air motion usually corresponds to anomalous high-pressure regions 44. Under the SAI scenario, an anomalous downward motion (red in Fig. 2f), indicating reduced upwelling over the longitudes of the core monsoon region, is found; this is also illustrated by the anomalous increase in geopotential height (here illustrated at 500 hPa, Fig. 3a) and sea-level pressure (Fig. 3c) over vast areas of India, Pakistan, and the Middle East. The anomalous subsidence of dry air over the subcontinent inhibits convection and rainfall over the Indian landmass. It also contributes to the anomalous warming at 850 hPa over large parts of Indian subcontinents (> 1ºC over the core monsoon region, Fig. 3b) to the reduction in adiabatic cooling. Additionally, slight anomalous upward motion (blue) over the longitudes of the Southern part of the Indian subcontinent (Fig. 3f) seems to support the increasing precipitation in that region. The nature of the phase of upper atmospheric wave activities and pressure velocity anomalies seems sufficient to explain the patterns of mean monsoon rainfall 53,56, as discussed in Section 1.
Other contributors to the reduction in rainfall simulated under SAI are possible. First, SAI-induced warming in the lower stratosphere (Fig. 2a) increases the static stability of the tropical troposphere 30,32, potentially inhibiting convection in the core Monsoon region (Fig. 2f). A similar mechanism has been proposed to explain the role of temperature anomalies associated with the different phases of the Quasi-Biennial Oscillation on the tropical convection in observations and idealized models 58,59. Second, the substantial reductions in the low-level wind speed at 850 hPa level over the Arabian Sea (anomalous easterly winds in Fig. 2e; compared with the climatology in Fig. S3b) prevents moisture convergence (Fig S4) to the mainland, resulting in a reduction of the mean Indian summer monsoon rainfall 44,60. Third, an anomalous northwesterly wind over north India and an anticyclonic feature over the monsoon trough region (over the head Bay of Bengal) do not allow the continental ITCZ to move northward 51, hindering the monsoon strength and moisture inflow from the Bay of Bengal branch.
Finally, past studies have reported that a global warming hiatus scenario could further weaken the pressure gradient between the Mascarene High and the northern hemisphere landmass 61. Our findings show similar results under the SAI scenario (Figure S5). Such weakening of Mascarene High intensity could have further weakened the high-level cross-equatorial winds in the western Indian Ocean and monsoon hydrology.
4.1 Cloud cover anomalies
Clouds play a crucial role in the energy and hydrological cycles of the Earth–-atmosphere system 62,63. High clouds dominate the SAM region during monsoon months, whereas low clouds are more frequent 64. For the SAI scenario, a significant and widespread reduction in low and high cloud cover is simulated over the Indian region. A notable reduction (> 5%) in high cloud cover is found over a large part of the Indian landmass aligned to the maximum rainfall reduction (Fig. 1). A similar signature is also observed in total cloud cover (Fig. 4c). On the contrary, the low cloud anomalies possess a spatial pattern (north-south dipole) similar to precipitation anomalies.
The moisture deficit over land, reduced convection, and the lower and mid-tropospheric anomalous high-pressure system are possible reasons behind such widespread reduction in cloud cover under the SAI scenario.